Attempting to Program Flash Memory on PYNQ Z1

Good morning,
I’m attempting to program the QSPI flash memory on the PYNQ Z1 with the ISSI IS43TR memory chip.
I have a default Verilog code that I want the PYNQ to work from at boot up and putting the Boot.bin on the SD card and running that has yielded no luck either, though I can program the device via JTAG without issue…

I’m not sure what to select in Vitis, or if there’s a better way to program the QSPI. I keep getting a “Problem running uboot. Flash programming initialization failed” error.